Melting of Charge Density Waves in Low Dimensions

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Abstract Charge density waves (CDWs) are collective electronic states that can reshape and melt, even while confined within a rigid atomic crystal. In two dimensions, melting is predicted to be distinct, proceeding through partially ordered nematic and hexatic states that are neither liquid nor crystal. Here we measure and explain how continuous, hexatic melting of incommensurate CDWs occurs in low-dimensional materials. As a CDW is thermally excited, disorder emerges progressively---initially through smooth elastic deformations that modulate the local wavelength, and subsequently via the nucleation of topological defects. Experimentally, we track three hallmark signatures of CDW melting---azimuthal superlattice peak broadening, wavevector contraction, and integrated intensity decay.
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Melting of Charge Density Waves in Low Dimensions | Research Square window.SnipcartSettings = { analytics: { enabled: false } }; (function() { var accessVector = localStorage.getItem('access_vector') || ''; window.dataLayer = window.dataLayer || []; if (accessVector) { window.dataLayer.push({ user: { profile: { profileInfo: { snid: accessVector } } } }); } })(); (function(w,d,s,l,i){w[l]=w[l]||[];w[l].push({'gtm.start':new Date().getTime(),event:'gtm.js'});var f=d.getElementsByTagName(s)[0],j=d.createElement(s),dl=l!='dataLayer'?'&l='+l:'';j.async=true;j.src='https://www.googletagmanager.com/gtm.js?id='+i+dl;f.parentNode.insertBefore(j,f);})(window,document,'script','dataLayer','GTM-K279D39R'); Browse Preprints In Review Journals COVID-19 Preprints AJE Video Bytes Research Tools Research Promotion AJE Professional Editing AJE Rubriq About Preprint Platform In Review Editorial Policies Our Team Advisory Board Help Center Sign In Submit a Preprint Cite Share Download PDF Physical Sciences - Article Melting of Charge Density Waves in Low Dimensions Robert Hovden, Jeremy Shen, Alex Stangel, Suk Hyun Sung, Nishkarsh Agarwal, and 2 more This is a preprint; it has not been peer reviewed by a journal. https://doi.org/ 10.21203/rs.3.rs-6614897/v1 This work is licensed under a CC BY 4.0 License Status: Posted Version 1 posted You are reading this latest preprint version Abstract Charge density waves (CDWs) are collective electronic states that can reshape and melt, even while confined within a rigid atomic crystal. In two dimensions, melting is predicted to be distinct, proceeding through partially ordered nematic and hexatic states that are neither liquid nor crystal. Here we measure and explain how continuous, hexatic melting of incommensurate CDWs occurs in low-dimensional materials. As a CDW is thermally excited, disorder emerges progressively---initially through smooth elastic deformations that modulate the local wavelength, and subsequently via the nucleation of topological defects. Experimentally, we track three hallmark signatures of CDW melting---azimuthal superlattice peak broadening, wavevector contraction, and integrated intensity decay. Physical sciences/Materials science/Techniques and instrumentation/Microscopy/Transmission electron microscopy Physical sciences/Materials science/Condensed-matter physics/Structure of solids and liquids Physical sciences/Physics/Condensed-matter physics/Electronic properties and materials Full Text Additional Declarations There is NO Competing Interest. Supplementary Files 2025CDWmeltingShenStangelSIvf.pdf 2025_CDW_Melting_ShenStangel_SI Cite Share Download PDF Status: Posted Version 1 posted You are reading this latest preprint version Research Square lets you share your work early, gain feedback from the community, and start making changes to your manuscript prior to peer review in a journal. As a division of Research Square Company, we’re committed to making research communication faster, fairer, and more useful. We do this by developing innovative software and high quality services for the global research community. Our growing team is made up of researchers and industry professionals working together to solve the most critical problems facing scientific publishing. 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