Highly Magneto-electric-mechanical Coupling Effect in Self-biased Magnetoelectric Composite Induced by Laser Thermal Annealing | Research Square window.SnipcartSettings = { analytics: { enabled: false } }; (function() { var accessVector = localStorage.getItem('access_vector') || ''; window.dataLayer = window.dataLayer || []; if (accessVector) { window.dataLayer.push({ user: { profile: { profileInfo: { snid: accessVector } } } }); } })(); (function(w,d,s,l,i){w[l]=w[l]||[];w[l].push({'gtm.start':new Date().getTime(),event:'gtm.js'});var f=d.getElementsByTagName(s)[0],j=d.createElement(s),dl=l!='dataLayer'?'&l='+l:'';j.async=true;j.src='https://www.googletagmanager.com/gtm.js?id='+i+dl;f.parentNode.insertBefore(j,f);})(window,document,'script','dataLayer','GTM-K279D39R'); Browse Preprints In Review Journals COVID-19 Preprints AJE Video Bytes Research Tools Research Promotion AJE Professional Editing AJE Rubriq About Preprint Platform In Review Editorial Policies Our Team Advisory Board Help Center Sign In Submit a Preprint Cite Share Download PDF Article Highly Magneto-electric-mechanical Coupling Effect in Self-biased Magnetoelectric Composite Induced by Laser Thermal Annealing Ming Liu, DAN XIAN, Yanan Zhao, Yongjun Du, Yiwei Xu, Jiacheng Qiao, and 3 more This is a preprint; it has not been peer reviewed by a journal. https://doi.org/ 10.21203/rs.3.rs-5235810/v1 This work is licensed under a CC BY 4.0 License Status: Published Journal Publication published 15 Jul, 2025 Read the published version in Microsystems & Nanoengineering → Version 1 posted 9 You are reading this latest preprint version Abstract The development of advanced magnetoelectric (ME) composites necessitates high-performance materials is capable of achieving high levels of ME coupling, minimal magnetic loss, absence or limited reliance on external excitation sources. In this paper, a (2-2) connectivity magnetoelectric (ME) laminate integrates multiple layers of FeSiB alloy (Metglas) and Pb (Mg, Nb) O3-PbTiO3 (PMN-PT) single crystal, achieving a remarkable ME coupling coefficient of 2033.4 V/Oe·cm (sevenfold rise) by laser thermal annealing treatment. Here, the laser-induced nanostructures on Metglas, with oxidized insulation layer and soft and hard magnetic dipole layer improve the Magneto-electric-mechanical coupling with a mechanical quality factor exceeding 350. More importantly, the interaction between amorphous and nanocrystalline dipoles triggers an EB effect, leading to self-biasing performance of 67.45 V/Oe·cm. Furthermore, the composite exhibits excellent passive DC magnetic detection limit of 22 nT, and an improved weak AC magnetic detection limit down to 383 fT. These explorations offer the potential to enhance passive current measurement, underwater communication, extend weak magnetic positioning, and extend brain magnetic detection. magnetoelectric coupling laser thermal annealing self-biased Full Text Additional Declarations (Not answered) Cite Share Download PDF Status: Published Journal Publication published 15 Jul, 2025 Read the published version in Microsystems & Nanoengineering → Version 1 posted Editorial decision: revise 14 Nov, 2024 Review # 2 received at journal 05 Nov, 2024 Reviewer # 2 agreed at journal 25 Oct, 2024 Review # 1 received at journal 22 Oct, 2024 Reviewer # 1 agreed at journal 15 Oct, 2024 Reviewers invited by journal 15 Oct, 2024 Submission checks completed at journal 10 Oct, 2024 Editor assigned by journal 09 Oct, 2024 First submitted to journal 09 Oct, 2024 You are reading this latest preprint version Research Square lets you share your work early, gain feedback from the community, and start making changes to your manuscript prior to peer review in a journal. As a division of Research Square Company, we’re committed to making research communication faster, fairer, and more useful. We do this by developing innovative software and high quality services for the global research community. Our growing team is made up of researchers and industry professionals working together to solve the most critical problems facing scientific publishing. Also discoverable on Platform About Our Team In Review Editorial Policies Advisory Board Help Center Resources Author Services Accessibility API Access RSS feed Manage Cookie Preferences © Research Square 2026 | ISSN 2693-5015 (online) Privacy Policy Terms of Service Do Not Sell My Personal Information {"props":{"pageProps":{"initialData":{"identity":"rs-5235810","acceptedTermsAndConditions":true,"allowDirectSubmit":false,"archivedVersions":[],"articleType":"Article","associatedPublications":[],"authors":[{"id":366305018,"identity":"add4d02f-efbe-4c1b-9def-f6fa3ab7b2df","order_by":0,"name":"Ming Liu","email":"data:image/png;base64,iVBORw0KGgoAAAANSUhEUgAAAZAAAAAyAQMAAABI0h/eAAAABlBMVEX///8AAABVwtN+AAAACXBIWXMAAA7EAAAOxAGVKw4bAAAA00lEQVRIie3RMQrCMBSA4SeFdql2zaKeQIgESqGXSRazqDg6OGSqY2dv4RFaAp0qXTvWzTEHEDGNuLYZBfNDKYH3UfIK4HL9Yp5+OgwLgOJ7tCEUAwGQtqSPAjDxmbYgq/NUPuhB8mvZVAiOKRPBrRgksZxtEorl7iKkj6DmTIR7OkLCGPckB00mmWQChdiKcN+Qlx0hnSY0MkRYfkUvma/1XUhCK06ycDtCmpoo9UyXuC3vrTql8zyoh4lOL6oPFeYHgT82r/OUeUXCYtblcrn+sjcvcUOaUT0D5wAAAABJRU5ErkJggg==","orcid":"","institution":"Xi'an Jiaotong University","correspondingAuthor":true,"submittingAuthor":false,"prefix":"","firstName":"Ming","middleName":"","lastName":"Liu","suffix":""},{"id":366305019,"identity":"39640d93-eb10-44d0-87ae-c77a96abb0d1","order_by":1,"name":"DAN XIAN","email":"","orcid":"","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"DAN","middleName":"","lastName":"XIAN","suffix":""},{"id":366305020,"identity":"56dc430e-1ec4-472c-a41e-fc8641de1bcc","order_by":2,"name":"Yanan Zhao","email":"","orcid":"","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Yanan","middleName":"","lastName":"Zhao","suffix":""},{"id":366305021,"identity":"c8d12606-dff4-4033-91d9-f138d0ee2bf7","order_by":3,"name":"Yongjun Du","email":"","orcid":"https://orcid.org/0000-0001-5006-2152","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Yongjun","middleName":"","lastName":"Du","suffix":""},{"id":366305022,"identity":"9e1880fb-0a20-45f6-98f2-878564ef0d94","order_by":4,"name":"Yiwei Xu","email":"","orcid":"https://orcid.org/0000-0001-8923-6113","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Yiwei","middleName":"","lastName":"Xu","suffix":""},{"id":366305023,"identity":"38b5480c-f42e-4151-aae2-fc9a217efd4a","order_by":5,"name":"Jiacheng Qiao","email":"","orcid":"https://orcid.org/0000-0003-0240-8547","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Jiacheng","middleName":"","lastName":"Qiao","suffix":""},{"id":366305024,"identity":"272623d2-17fd-49e1-a3f9-3c9e9d8b7ca2","order_by":6,"name":"Jingen Wu","email":"","orcid":"","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Jingen","middleName":"","lastName":"Wu","suffix":""},{"id":366305025,"identity":"e890c3e2-670a-4d52-abde-6398115ddabd","order_by":7,"name":"Qijing Lin","email":"","orcid":"","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Qijing","middleName":"","lastName":"Lin","suffix":""},{"id":366305026,"identity":"fc6b4896-427e-4f66-a4fb-ea6044a7341a","order_by":8,"name":"Zhuangde Jiang","email":"","orcid":"","institution":"Xi'an Jiaotong University","correspondingAuthor":false,"submittingAuthor":false,"prefix":"","firstName":"Zhuangde","middleName":"","lastName":"Jiang","suffix":""}],"badges":[],"createdAt":"2024-10-10 02:40:15","currentVersionCode":1,"declarations":"","doi":"10.21203/rs.3.rs-5235810/v1","doiUrl":"https://doi.org/10.21203/rs.3.rs-5235810/v1","draftVersion":[],"editorialEvents":[{"content":"https://doi.org/10.1038/s41378-025-00875-w","type":"published","date":"2025-07-15T04:00:00+00:00"}],"editorialNote":"","failedWorkflow":false,"files":[{"id":86742705,"identity":"7491175f-686e-4c56-8f88-94ee0bbd8a87","added_by":"auto","created_at":"2025-07-15 07:13:46","extension":"pdf","order_by":1,"title":"","display":"","copyAsset":false,"role":"manuscript-pdf","size":968300,"visible":true,"origin":"","legend":"Article File","description":"","filename":"manuscript.pdf","url":"https://assets-eu.researchsquare.com/files/rs-5235810/v1_covered_f129fd03-9eed-4275-accf-a6c2028fc62c.pdf"}],"financialInterests":"(Not answered)","formattedTitle":"Highly Magneto-electric-mechanical Coupling Effect in Self-biased Magnetoelectric Composite Induced by Laser Thermal Annealing","fulltext":[],"fulltextSource":"","fullText":"","funders":[],"hasAdminPriorityOnWorkflow":false,"hasManuscriptDocX":false,"hasOptedInToPreprint":true,"hasPassedJournalQc":"","hasAnyPriority":false,"hideJournal":false,"highlight":"","institution":"","isAcceptedByJournal":true,"isAuthorSuppliedPdf":true,"isDeskRejected":"","isHiddenFromSearch":false,"isInQc":false,"isInWorkflow":false,"isPdf":true,"isPdfUpToDate":true,"isWithdrawnOrRetracted":false,"journal":{"display":true,"email":"
[email protected]","identity":"microsystems-and-nanoengineering","isNatureJournal":false,"hasQc":false,"allowDirectSubmit":false,"externalIdentity":"micronano","sideBox":"Learn more about [Microsystems \u0026 Nanoengineering](http://www.nature.com/micronano/)","snPcode":"41378","submissionUrl":"https://mts-micronano.nature.com/","title":"Microsystems \u0026 Nanoengineering","twitterHandle":"","acdcEnabled":true,"dfaEnabled":true,"editorialSystem":"ejp","reportingPortfolio":"Nature AJ","inReviewEnabled":true,"inReviewRevisionsEnabled":true},"keywords":"magnetoelectric coupling, laser thermal annealing, self-biased","lastPublishedDoi":"10.21203/rs.3.rs-5235810/v1","lastPublishedDoiUrl":"https://doi.org/10.21203/rs.3.rs-5235810/v1","license":{"name":"CC BY 4.0","url":"https://creativecommons.org/licenses/by/4.0/"},"manuscriptAbstract":"The development of advanced magnetoelectric (ME) composites necessitates high-performance materials is capable of achieving high levels of ME coupling, minimal magnetic loss, absence or limited reliance on external excitation sources. In this paper, a (2-2) connectivity magnetoelectric (ME) laminate integrates multiple layers of FeSiB alloy (Metglas) and Pb (Mg, Nb) O3-PbTiO3 (PMN-PT) single crystal, achieving a remarkable ME coupling coefficient of 2033.4 V/Oe·cm (sevenfold rise) by laser thermal annealing treatment. Here, the laser-induced nanostructures on Metglas, with oxidized insulation layer and soft and hard magnetic dipole layer improve the Magneto-electric-mechanical coupling with a mechanical quality factor exceeding 350. More importantly, the interaction between amorphous and nanocrystalline dipoles triggers an EB effect, leading to self-biasing performance of 67.45 V/Oe·cm. Furthermore, the composite exhibits excellent passive DC magnetic detection limit of 22 nT, and an improved weak AC magnetic detection limit down to 383 fT. These explorations offer the potential to enhance passive current measurement, underwater communication, extend weak magnetic positioning, and extend brain magnetic detection.","manuscriptTitle":"Highly Magneto-electric-mechanical Coupling Effect in Self-biased Magnetoelectric Composite Induced by Laser Thermal Annealing","msid":"","msnumber":"","nonDraftVersions":[{"code":1,"date":"2024-10-17 06:45:03","doi":"10.21203/rs.3.rs-5235810/v1","editorialEvents":[{"type":"communityComments","content":0},{"type":"decision","content":"revise","date":"2024-11-14T08:51:30+00:00","index":"","fulltext":""},{"type":"editorInvitedReview","content":"This content is not available.","date":"2024-11-05T12:08:31+00:00","index":2,"fulltext":"This content is not available."},{"type":"reviewerAgreed","content":"This content is not available.","date":"2024-10-25T04:48:55+00:00","index":2,"fulltext":"This content is not available."},{"type":"editorInvitedReview","content":"This content is not available.","date":"2024-10-22T10:59:39+00:00","index":1,"fulltext":"This content is not available."},{"type":"reviewerAgreed","content":"This content is not available.","date":"2024-10-16T01:59:21+00:00","index":1,"fulltext":"This content is not available."},{"type":"reviewersInvited","content":"","date":"2024-10-15T12:44:21+00:00","index":"","fulltext":""},{"type":"checksComplete","content":"","date":"2024-10-10T11:20:13+00:00","index":"","fulltext":""},{"type":"editorAssigned","content":"","date":"2024-10-10T02:38:36+00:00","index":"","fulltext":""},{"type":"submitted","content":"Microsystems \u0026 Nanoengineering","date":"2024-10-10T02:38:35+00:00","index":"","fulltext":""}],"status":"published","journal":{"display":true,"email":"
[email protected]","identity":"microsystems-and-nanoengineering","isNatureJournal":false,"hasQc":false,"allowDirectSubmit":false,"externalIdentity":"micronano","sideBox":"Learn more about [Microsystems \u0026 Nanoengineering](http://www.nature.com/micronano/)","snPcode":"41378","submissionUrl":"https://mts-micronano.nature.com/","title":"Microsystems \u0026 Nanoengineering","twitterHandle":"","acdcEnabled":true,"dfaEnabled":true,"editorialSystem":"ejp","reportingPortfolio":"Nature AJ","inReviewEnabled":true,"inReviewRevisionsEnabled":true}}],"origin":"","ownerIdentity":"b6cb5742-826e-482e-b750-c9116c77370e","owner":[],"postedDate":"October 17th, 2024","published":true,"recentEditorialEvents":[],"rejectedJournal":[],"revision":"","amendment":"","status":"published-in-journal","subjectAreas":[],"tags":[],"updatedAt":"2025-07-15T07:13:41+00:00","versionOfRecord":{"articleIdentity":"rs-5235810","link":"https://doi.org/10.1038/s41378-025-00875-w","journal":{"identity":"microsystems-and-nanoengineering","isVorOnly":false,"title":"Microsystems \u0026 Nanoengineering"},"publishedOn":"2025-07-15 04:00:00","publishedOnDateReadable":"July 15th, 2025"},"versionCreatedAt":"2024-10-17 06:45:03","video":"","vorDoi":"10.1038/s41378-025-00875-w","vorDoiUrl":"https://doi.org/10.1038/s41378-025-00875-w","workflowStages":[]},"version":"v1","identity":"rs-5235810","journalConfig":"researchsquare"},"__N_SSP":true},"page":"/article/[identity]/[[...version]]","query":{"redirect":"/article/rs-5235810","identity":"rs-5235810","version":["v1"]},"buildId":"7rjqhiLT3MXkJMwkYKINL","isFallback":false,"isExperimentalCompile":false,"dynamicIds":[84888],"gssp":true,"scriptLoader":[]}
Text is read by the "Ask this paper" AI Q&A widget below.
Extraction quality varies by source — PMC NXML preserves structure
cleanly, OA-HTML may include some navigation residue, and OA-PDF can
have broken hyphenation. The publisher copy
(via DOI)
is the canonical version.