Spin Wave Spectra in Pseudoperovskite Manganites with Superexchange Interaction Competition

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This study calculates spin-wave dispersion dependences in pseudoperovskite manganites, revealing frustrated spectra with crossing and splitting of branches due to competing superexchange interactions and anisotropy.

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The paper calculates spin-wave dispersion relations in the pseudoperovskite manganites La1/3Ca2/3MnO3 and BiMnO3 by modeling orbitally dependent nearest-neighbor superexchange interactions and single-ion anisotropy within a regular multi-sublattice framework. It considers how orbital or charge-orbital ordering leads to competing exchange interactions inside the magnetic unit cell, producing frustrated spin-wave spectra. The key results are that crossing and splitting of spin-wave branches occur commonly at non-symmetric points of the magnetic Brillouin zone due to exchange competition, and it predicts the Γ-point spin-wave band structure for both compounds. The study is limited to the theoretical nearest-neighbor superexchange and the specified modeling assumptions rather than direct experimental validation. The paper does not explicitly discuss endometriosis or adenomyosis; it was included in the corpus via a keyword match in the upstream search index.

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Abstract

In compounds La 1/3 Ca 2/3 MnO 3 and BiMnO 3 , a calculation of spin-wave dispersion dependences along pseudoperovskite directions of reciprocal space is made. The model includes orbitally-dependent superexchange interaction and single-ion anisotropy. Considered compounds present competing exchange interactions within magnetic unit cell because of orbital or charge-orbital ordering. The nearest neighbor superexchange interaction is taken into account. The magnetic structure and dispersion dependences of spin waves frequencies are calculated within the framework of regular multi-sublattice model. The peculiarities of frustrated magnetic spin-wave spectra are found. It is shown, that crossing and splitting of spin-waves branches in non-symmetric points of magnetic Brillouin zone is a common feature of the spectra due to exchange competition. The band structure of Γ-point spectra for both compounds are predicted.
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Spin Wave Spectra in Pseudoperovskite Manganites with Superexchange Interaction Competition | Research Square window.SnipcartSettings = { analytics: { enabled: false } }; (function() { var accessVector = localStorage.getItem('access_vector') || ''; window.dataLayer = window.dataLayer || []; if (accessVector) { window.dataLayer.push({ user: { profile: { profileInfo: { snid: accessVector } } } }); } })(); (function(w,d,s,l,i){w[l]=w[l]||[];w[l].push({'gtm.start':new Date().getTime(),event:'gtm.js'});var f=d.getElementsByTagName(s)[0],j=d.createElement(s),dl=l!='dataLayer'?'&l='+l:'';j.async=true;j.src='https://www.googletagmanager.com/gtm.js?id='+i+dl;f.parentNode.insertBefore(j,f);})(window,document,'script','dataLayer','GTM-K279D39R'); Browse Preprints In Review Journals COVID-19 Preprints AJE Video Bytes Research Tools Research Promotion AJE Professional Editing AJE Rubriq About Preprint Platform In Review Editorial Policies Our Team Advisory Board Help Center Sign In Submit a Preprint Cite Share Download PDF Research Article Spin Wave Spectra in Pseudoperovskite Manganites with Superexchange Interaction Competition Liudmila E. Gonchar This is a preprint; it has not been peer reviewed by a journal. https://doi.org/ 10.21203/rs.3.rs-2397192/v1 This work is licensed under a CC BY 4.0 License Status: Published Journal Publication published 15 Mar, 2023 Read the published version in Applied Magnetic Resonance → Version 1 posted 7 You are reading this latest preprint version Abstract In compounds La 1/3 Ca 2/3 MnO 3 and BiMnO 3 , a calculation of spin-wave dispersion dependences along pseudoperovskite directions of reciprocal space is made. The model includes orbitally-dependent superexchange interaction and single-ion anisotropy. Considered compounds present competing exchange interactions within magnetic unit cell because of orbital or charge-orbital ordering. The nearest neighbor superexchange interaction is taken into account. The magnetic structure and dispersion dependences of spin waves frequencies are calculated within the framework of regular multi-sublattice model. The peculiarities of frustrated magnetic spin-wave spectra are found. It is shown, that crossing and splitting of spin-waves branches in non-symmetric points of magnetic Brillouin zone is a common feature of the spectra due to exchange competition. The band structure of Γ-point spectra for both compounds are predicted. manganites orbitally-dependent superexchange multi-sublattice magnetic structure spin excitations Full Text Additional Declarations No competing interests reported. Cite Share Download PDF Status: Published Journal Publication published 15 Mar, 2023 Read the published version in Applied Magnetic Resonance → Version 1 posted Editorial decision: Major revision 09 Jan, 2023 Reviews received at journal 28 Dec, 2022 Reviewers agreed at journal 25 Dec, 2022 Reviewers invited by journal 24 Dec, 2022 Editor assigned by journal 23 Dec, 2022 Submission checks completed at journal 22 Dec, 2022 First submitted to journal 20 Dec, 2022 You are reading this latest preprint version Research Square lets you share your work early, gain feedback from the community, and start making changes to your manuscript prior to peer review in a journal. As a division of Research Square Company, we’re committed to making research communication faster, fairer, and more useful. We do this by developing innovative software and high quality services for the global research community. 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