Comparative Analysis of Simplified and Extended Chemistry Models in Low-Pressure Argon DC Discharge

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This study found that a simplified chemistry model overestimates plasma density and discharge current in low-pressure argon DC discharges compared to a more detailed model, highlighting the necessity of accounting for excited level structures.

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The paper studies how plasma-chemical reaction assumptions affect fluid modeling results for a low-pressure (1 Torr) argon DC glow discharge, comparing a Simplified Chemistry Model that uses one lumped excited level versus an Extended Chemistry Model that separates metastable and resonance states and includes resonance radiation transport. The authors find that using the simplified approach overestimates plasma density by a factor of 2–3 and discharge current by about 23% relative to the more detailed model. They report that neglecting radiative losses from resonance levels breaks energy and particle balance and leads to inaccurate predictions even at low pressure, with ionization-rate analysis showing an artificial overestimation of stepwise ionization in the simplified model. This paper does not explicitly discuss endometriosis or adenomyosis; it was included in the corpus via a keyword match in the upstream search index.

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Abstract

Abstract In the present work, a comparative study of the influence of plasma-chemical reactions on the results of fluid modeling of a direct current (DC) glow discharge in argon at a pressure of 1 Torr is presented. Here two approaches are compared: a Simplified Chemistry Model (SCM), which accounts for only one lumped excited level, and an Extended Chemistry Model (ECM), in which metastable and resonance states are explicitly separated, and resonance radiation transport is taken into account. The use of SCM leads to an overestimation of plasma density (by a factor of 2-3) and discharge current (by ~23%) compared to the more detailed ECM. It is shown that neglecting radiative losses from resonance levels in simplified models violates the energy and particle balance, leading to inaccurate predictions even at low pressures. Analysis of ionization rates demonstrates that the simplified model artificially overestimates the contribution of stepwise ionization. The results demonstrate the necessity of accounting for the detailed structure of excited levels for quantitatively accurate modeling of gas discharge devices even at low pressures.
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Comparative Analysis of Simplified and Extended Chemistry Models in Low-Pressure Argon DC Discharge | Research Square window.SnipcartSettings = { analytics: { enabled: false } }; (function() { var accessVector = localStorage.getItem('access_vector') || ''; window.dataLayer = window.dataLayer || []; if (accessVector) { window.dataLayer.push({ user: { profile: { profileInfo: { snid: accessVector } } } }); } })(); (function(w,d,s,l,i){w[l]=w[l]||[];w[l].push({'gtm.start':new Date().getTime(),event:'gtm.js'});var f=d.getElementsByTagName(s)[0],j=d.createElement(s),dl=l!='dataLayer'?'&l='+l:'';j.async=true;j.src='https://www.googletagmanager.com/gtm.js?id='+i+dl;f.parentNode.insertBefore(j,f);})(window,document,'script','dataLayer','GTM-K279D39R'); Browse Preprints In Review Journals COVID-19 Preprints AJE Video Bytes Research Tools Research Promotion AJE Professional Editing AJE Rubriq About Preprint Platform In Review Editorial Policies Our Team Advisory Board Help Center Sign In Submit a Preprint Cite Share Download PDF Research Article Comparative Analysis of Simplified and Extended Chemistry Models in Low-Pressure Argon DC Discharge Kurban M Rabadanov, Gadzhi Sh Shakhsinov This is a preprint; it has not been peer reviewed by a journal. https://doi.org/ 10.21203/rs.3.rs-9184005/v1 This work is licensed under a CC BY 4.0 License Status: Posted Version 1 posted You are reading this latest preprint version Abstract In the present work, a comparative study of the influence of plasma-chemical reactions on the results of fluid modeling of a direct current (DC) glow discharge in argon at a pressure of 1 Torr is presented. Here two approaches are compared: a Simplified Chemistry Model (SCM), which accounts for only one lumped excited level, and an Extended Chemistry Model (ECM), in which metastable and resonance states are explicitly separated, and resonance radiation transport is taken into account. The use of SCM leads to an overestimation of plasma density (by a factor of 2-3) and discharge current (by ~23%) compared to the more detailed ECM. It is shown that neglecting radiative losses from resonance levels in simplified models violates the energy and particle balance, leading to inaccurate predictions even at low pressures. Analysis of ionization rates demonstrates that the simplified model artificially overestimates the contribution of stepwise ionization. The results demonstrate the necessity of accounting for the detailed structure of excited levels for quantitatively accurate modeling of gas discharge devices even at low pressures. Gas-discharge direct current discharge argon plasma low-pressure plasma numerical simulation Full Text Additional Declarations No competing interests reported. Cite Share Download PDF Status: Posted Version 1 posted You are reading this latest preprint version Research Square lets you share your work early, gain feedback from the community, and start making changes to your manuscript prior to peer review in a journal. As a division of Research Square Company, we’re committed to making research communication faster, fairer, and more useful. We do this by developing innovative software and high quality services for the global research community. Our growing team is made up of researchers and industry professionals working together to solve the most critical problems facing scientific publishing. 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