On the Complex Dielectric, Complex Electric Modulus, and Conductivity of Au/(Brushite + Monetite: Pvc)/n-si (Mps) Structures in the Wide Range of Frequency and Voltage

On the Complex Dielectric, Complex Electric Modulus, and Conductivity of Au/(Brushite + Monetite: Pvc)/n-si (Mps) Structures in the Wide Range of Frequency and Voltage | Research Square window.SnipcartSettings = { analytics: { enabled: false } }; (function() { var accessVector = localStorage.getItem('access_vector') || ''; window.dataLayer = window.dataLayer || []; if (accessVector) { window.dataLayer.push({ user: { profile: { profileInfo: { snid: accessVector } } } }); } })(); (function(w,d,s,l,i){w[l]=w[l]||[];w[l].push({'gtm.start':new Date().getTime(),event:'gtm.js'});var f=d.getElementsByTagName(s)[0],j=d.createElement(s),dl=l!='dataLayer'?'&l='+l:'';j.async=true;j.src='https://www.googletagmanager.com/gtm.js?id='+i+dl;f.parentNode.insertBefore(j,f);})(window,document,'script','dataLayer','GTM-K279D39R'); Browse Preprints In Review Journals COVID-19 Preprints AJE Video Bytes Research Tools Research Promotion AJE Professional Editing AJE Rubriq About Preprint Platform In Review Editorial Policies Our Team Advisory Board Help Center Sign In Submit a Preprint Cite Share Download PDF Research Article On the Complex Dielectric, Complex Electric Modulus, and Conductivity of Au/(Brushite + Monetite: Pvc)/n-si (Mps) Structures in the Wide Range of Frequency and Voltage ŞEVKET ULUTÜRK, GÜLÇİN ERSÖZ DEMİR, ŞEMSETTİN ALTINDAL, İBRAHİM YÜCEDAĞ, and 2 more This is a preprint; it has not been peer reviewed by a journal. https://doi.org/ 10.21203/rs.3.rs-8997855/v1 This work is licensed under a CC BY 4.0 License Status: Posted Version 1 posted You are reading this latest preprint version Abstract This study investigates the complex interplay between dielectric properties and the Au/(B + M-doped PVC)/n-Si organic interlayer within metal-polymer-semiconductor (MPS) structures. The work aims to comprehensively analyze the (B + M:PVC)'s impact on MPS dielectric, electric modulus, and conductivity properties, contributing to a deeper understanding of nanoscale materials in electronic devices. Impedance measurements of Au/n-Si Schottky structures with (B + M-doped PVC) composite-interlayer were conducted across a wide range of frequencies (2kHz-2MHz) and voltages (-3V/+4V). The exploration uncovers frequency-voltage dependence on crucial parameters like loss tangent ( tanδ ), complex permittivity ( ɛ* ), AC electrical conductivity ( σ ac ), and complex electrical modulus ( M* ). Meanwhile, capacitance-conductance ( C-G/ω ) measurements were utilized to derive the graphs for ɛ' , ɛ” , M' , M'' , Z' , Z'' , σ ac , and tanδ in relation to frequency and voltage variations. The interface states and polarization are effective at low and medium frequencies in both the reversal and depletion regions. In contrast, at high frequencies, the series resistance is effective only in the accumulation region. The obtained high dielectric interlayer ( ɛ' = 14,25) even at 2 kHz indicates that this organic interlayer can be successfully used in electronic devices instead of conventional insulators/oxides in terms of low cost/weight, easy performance, flexibility, high dynamic strength, and high energy storage capacity. (Brushite+Monetite: PVC) organic interlayer Frequency and voltage dependence Dielectric electrical modulus and ac conductivity Interface traps and polarization processes Full Text Additional Declarations No competing interests reported. Cite Share Download PDF Status: Posted Version 1 posted You are reading this latest preprint version Research Square lets you share your work early, gain feedback from the community, and start making changes to your manuscript prior to peer review in a journal. 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Voltage\u003c/p\u003e","fulltext":[],"fulltextSource":"","fullText":"","funders":[],"hasAdminPriorityOnWorkflow":false,"hasManuscriptDocX":false,"hasOptedInToPreprint":true,"hasPassedJournalQc":"","hasAnyPriority":false,"hideJournal":true,"highlight":"","institution":"","isAcceptedByJournal":false,"isAuthorSuppliedPdf":true,"isDeskRejected":"","isHiddenFromSearch":false,"isInQc":false,"isInWorkflow":false,"isPdf":true,"isPdfUpToDate":true,"isWithdrawnOrRetracted":false,"journal":{"display":true,"email":"[email protected]","identity":"researchsquare","isNatureJournal":false,"hasQc":true,"allowDirectSubmit":true,"externalIdentity":"","sideBox":"","snPcode":"","submissionUrl":"/submission","title":"Research Square","twitterHandle":"researchsquare","acdcEnabled":true,"dfaEnabled":false,"editorialSystem":"","reportingPortfolio":"","inReviewEnabled":false,"inReviewRevisionsEnabled":true},"keywords":"(Brushite+Monetite: PVC) organic interlayer, Frequency and voltage dependence, Dielectric, electrical modulus and ac conductivity, Interface traps and polarization processes","lastPublishedDoi":"10.21203/rs.3.rs-8997855/v1","lastPublishedDoiUrl":"https://doi.org/10.21203/rs.3.rs-8997855/v1","license":{"name":"CC BY 4.0","url":"https://creativecommons.org/licenses/by/4.0/"},"manuscriptAbstract":"\u003cp\u003eThis study investigates the complex interplay between dielectric properties and the Au/(B\u0026thinsp;+\u0026thinsp;M-doped PVC)/n-Si organic interlayer within metal-polymer-semiconductor (MPS) structures. The work aims to comprehensively analyze the (B\u0026thinsp;+\u0026thinsp;M:PVC)'s impact on MPS dielectric, electric modulus, and conductivity properties, contributing to a deeper understanding of nanoscale materials in electronic devices. Impedance measurements of Au/n-Si Schottky structures with (B\u0026thinsp;+\u0026thinsp;M-doped PVC) composite-interlayer were conducted across a wide range of frequencies (2kHz-2MHz) and voltages (-3V/+4V). The exploration uncovers frequency-voltage dependence on crucial parameters like loss tangent (\u003cem\u003etanδ\u003c/em\u003e), complex permittivity (\u003cem\u003eɛ*\u003c/em\u003e), AC electrical conductivity (\u003cem\u003eσ\u003c/em\u003e\u003csub\u003e\u003cem\u003eac\u003c/em\u003e\u003c/sub\u003e), and complex electrical modulus (\u003cem\u003eM*\u003c/em\u003e). Meanwhile, capacitance-conductance (\u003cem\u003eC-G/ω\u003c/em\u003e) measurements were utilized to derive the graphs for \u003cem\u003eɛ'\u003c/em\u003e, \u003cem\u003eɛ\u0026rdquo;\u003c/em\u003e, \u003cem\u003eM'\u003c/em\u003e, \u003cem\u003eM''\u003c/em\u003e, \u003cem\u003eZ'\u003c/em\u003e, \u003cem\u003eZ''\u003c/em\u003e, \u003cem\u003eσ\u003c/em\u003e\u003csub\u003e\u003cem\u003eac\u003c/em\u003e\u003c/sub\u003e, and tanδ in relation to frequency and voltage variations. The interface states and polarization are effective at low and medium frequencies in both the reversal and depletion regions. In contrast, at high frequencies, the series resistance is effective only in the accumulation region. The obtained high dielectric interlayer (\u003cem\u003eɛ'\u003c/em\u003e = 14,25) even at 2 kHz indicates that this organic interlayer can be successfully used in electronic devices instead of conventional insulators/oxides in terms of low cost/weight, easy performance, flexibility, high dynamic strength, and high energy storage capacity.\u003c/p\u003e","manuscriptTitle":"On the Complex Dielectric, Complex Electric Modulus, and Conductivity of Au/(Brushite + Monetite: Pvc)/n-si (Mps) Structures in the Wide Range of Frequency and Voltage","msid":"","msnumber":"","nonDraftVersions":[{"code":1,"date":"2026-03-23 22:14:23","doi":"10.21203/rs.3.rs-8997855/v1","editorialEvents":[{"type":"communityComments","content":0}],"status":"published","journal":{"display":true,"email":"[email protected]","identity":"researchsquare","isNatureJournal":false,"hasQc":true,"allowDirectSubmit":true,"externalIdentity":"","sideBox":"","snPcode":"","submissionUrl":"/submission","title":"Research Square","twitterHandle":"researchsquare","acdcEnabled":true,"dfaEnabled":false,"editorialSystem":"","reportingPortfolio":"","inReviewEnabled":false,"inReviewRevisionsEnabled":true}}],"origin":"","ownerIdentity":"1fd7197f-793e-40cb-8286-634569964f6d","owner":[],"postedDate":"March 23rd, 2026","published":true,"recentEditorialEvents":[],"rejectedJournal":[],"revision":"","amendment":"","status":"posted","subjectAreas":[],"tags":[],"updatedAt":"2026-04-14T08:10:19+00:00","versionOfRecord":[],"versionCreatedAt":"2026-03-23 22:14:23","video":"","vorDoi":"","vorDoiUrl":"","workflowStages":[]},"version":"v1","identity":"rs-8997855","journalConfig":"researchsquare"},"__N_SSP":true},"page":"/article/[identity]/[[...version]]","query":{"redirect":"/article/rs-8997855","identity":"rs-8997855","version":["v1"]},"buildId":"XKTyCvWXoU3ODBz1xrDgd","isFallback":false,"isExperimentalCompile":false,"dynamicIds":[84888],"gssp":true,"scriptLoader":[]}