Quantum transitions in 3He adsorbed on carbon nanotube

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Abstract

Abstract In gases adsorbed on smooth surfaces, the binding energy E 1 of the lowest quantum state (first layer) is usually much lower than that of the excited state (second layer), E 2 . The typical energy difference for helium on graphite amounts to about 50 K which gives a vanishingly small Boltzmann factor e -(E 2 -E 1 )/k B T at temperatures below 1 K, and no atom should be present on the excited level (second layer), according to statistical physics. However, in our investigations on sub-monolayer of 3 He adsorbed on a carbon nanotube, we have detected helium atoms traveling freely along the tube. Free particles were shown to be responsible for quantized satellite peaks appearing in mechanical oscillation spectra next to the main resonance. We demonstrate that side peaks reflect transitions between different longitudinal quantum states of free helium atoms on the oscillating tube. Radial quantum fluctuations in AC electric field have been considered in the framework of Rabi oscillations and shown to lift some amount of particles above the dense first layer. Besides, zero-point pressure at moderate densities promotes radial fluctuations significantly.
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Quantum transitions in 3He adsorbed on carbon nanotube | Research Square window.SnipcartSettings = { analytics: { enabled: false } }; (function() { var accessVector = localStorage.getItem('access_vector') || ''; window.dataLayer = window.dataLayer || []; if (accessVector) { window.dataLayer.push({ user: { profile: { profileInfo: { snid: accessVector } } } }); } })(); (function(w,d,s,l,i){w[l]=w[l]||[];w[l].push({'gtm.start':new Date().getTime(),event:'gtm.js'});var f=d.getElementsByTagName(s)[0],j=d.createElement(s),dl=l!='dataLayer'?'&l='+l:'';j.async=true;j.src='https://www.googletagmanager.com/gtm.js?id='+i+dl;f.parentNode.insertBefore(j,f);})(window,document,'script','dataLayer','GTM-K279D39R'); Browse Preprints In Review Journals COVID-19 Preprints AJE Video Bytes Research Tools Research Promotion AJE Professional Editing AJE Rubriq About Preprint Platform In Review Editorial Policies Our Team Advisory Board Help Center Sign In Submit a Preprint Cite Share Download PDF Article Quantum transitions in 3 He adsorbed on carbon nanotube Igor Todoshchenko, Masahiro Kamada, Jukka-Pekka Kaikkonen, Yongping Liao, and 6 more This is a preprint; it has not been peer reviewed by a journal. https://doi.org/ 10.21203/rs.3.rs-9276646/v1 This work is licensed under a CC BY 4.0 License Status: Under Review Version 1 posted You are reading this latest preprint version Abstract In gases adsorbed on smooth surfaces, the binding energy E 1 of the lowest quantum state (first layer) is usually much lower than that of the excited state (second layer), E 2 . The typical energy difference for helium on graphite amounts to about 50 K which gives a vanishingly small Boltzmann factor e -(E 2 -E 1 )/k B T at temperatures below 1 K, and no atom should be present on the excited level (second layer), according to statistical physics. However, in our investigations on sub-monolayer of 3 He adsorbed on a carbon nanotube, we have detected helium atoms traveling freely along the tube. Free particles were shown to be responsible for quantized satellite peaks appearing in mechanical oscillation spectra next to the main resonance. We demonstrate that side peaks reflect transitions between different longitudinal quantum states of free helium atoms on the oscillating tube. Radial quantum fluctuations in AC electric field have been considered in the framework of Rabi oscillations and shown to lift some amount of particles above the dense first layer. Besides, zero-point pressure at moderate densities promotes radial fluctuations significantly. Physical sciences/Physics/Quantum physics Physical sciences/Physics/Condensed-matter physics Full Text Additional Declarations There is NO Competing Interest. Supplementary Files CNTDISSIPATION27032026SUPPL.pdf Quantum transitions in 3 He adsorbed on carbon nanotube -- Supplementary Information Cite Share Download PDF Status: Under Review Version 1 posted You are reading this latest preprint version Research Square lets you share your work early, gain feedback from the community, and start making changes to your manuscript prior to peer review in a journal. As a division of Research Square Company, we’re committed to making research communication faster, fairer, and more useful. We do this by developing innovative software and high quality services for the global research community. Our growing team is made up of researchers and industry professionals working together to solve the most critical problems facing scientific publishing. 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